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Circular-dichroism in band dispersions and Fermi surfaces of Platinum metal : Connection with ‘spin’ and ‘orbital’ Hall conductivity

Dr. Ashish Chainani
Ashish Chainani
RIKEN Harima Institute at Spring-8, Hyogo-679-5148, Japan

2013年5月8日 13時30分 理学館506

We study the three-dimensional (3D) momentum-resolved electronic structure of bulk Platinum metal, which is known to show the largest ‘spin-Hall conductivity’ of all materials[1]. We measure circular-dichroism in the valence band dispersions and Fermi surfaces using soft x-ray angle resolved photoemission spectroscopy. The experimentally measured band dispersions and Fermi surfaces are consistent with band structure calculations including spin-orbit coupling[2]. However, the hexagonal Fermi surface around L point which shows negligible effects due to spin-orbit coupling, exhibits a large oscillatory circular dichroism with a period of 2π/3 radians. In contrast, the three lobe-shaped Fermi surfaces around L point derived from strong spin-orbit coupled states, show circular dichroism with a periodicity of 2π radians. The observed Fermi surface dependent circular dichroism can be associated with the theoretically known ‘orbital-Hall’ and ‘spin-Hall’ conductivity components[3]. We propose that the momentum dependent circular dichroism on the Fermi surfaces tracks the effective Aharonov-Bohm phase due to ‘orbital’ and ‘pseudo-spin’ texture in bulk Platinum metal, respectively.

This work is done in collaboration with J.Miyawaki, Y. Takata, M. Oura, Y. Senba, H. Ohashi, S. Shin, G. Y. Guo, B. Gu, S. Maekawa and N. Nagaosa.